| 1 | I Am a Rock | Paul Simon | 2:41 |
| 2 | Leaves That Are Green | Paul Simon | 2:31 |
| 3 | A Church Is Burning | Paul Simon | 3:23 |
| 4 | April Come She Will | Paul Simon | 1:48 |
| 5 | The Sound of Silence | Paul Simon | 3:06 |
| 6 | A Most Peculiar Man | Paul Simon | 2:24 |
| 7 | He Was My Brother | Paul Simon | 2:46 |
| 8 | Kathy's Song | Paul Simon | 3:28 |
| 9 | The Side of a Hill | Paul Simon | 2:18 |
| 10 | A Simple Desultory Philippic (Or How I Was Robert McNamara’d Into Submission) | Paul Simon | 2:18 |
| 11 | Flowers Never Bend With the Rainfall | Paul Simon | 2:18 |
| 12 | Patterns | Paul Simon | 3:03 |
| 13 | Carlos Dominguez (Paul Kane single - 1964) | Paul Simon | 2:44 |
| 14 | You Don't Know Where Your Interest Lies | Paul Simon | 2:21 |
| 15 | Overs (early demo take 14 -1966) | Paul Simon | 2:13 |
| 16 | For Emily, Wherever I May Find Her | Paul Simon | 2:05 |
| 17 | Silent Night | Paul Simon | 1:59 |
| 18 | The Star Carol | Paul Simon | 1:44 |
| 19 | The Sound of Silence (From "The Graduate") | Paul Simon | 3:07 |
| 20 | Mrs. Robinson (From "The Graduate") | Paul Simon | 1:10 |
| 21 | Homeward Bound (live - Greatest Hits) | Paul Simon | 2:43 |
| 22 | The 59th Street Bridge Song (live - Greatest Hits) | Paul Simon | 1:49 |
| 23 | For Emily, Wherever I May Find Her | Paul Simon | 2:21 |
| 24 | Kathy's Song (live - Greatest Hits) | Paul Simon | 3:22 |
| 25 | Bridge Over Troubled Water (Solo demo - 1969) | Paul Simon | 2:35 |
| 26 | Homeward Bound (w/ Harrison From SNL) | Paul Simon | 2:40 |
| 27 | What a Wonderful World | Paul Simon | 3:24 |
| 28 | Song About the Moon | Paul Simon | 3:58 |