| 1 | Prelude: Thoroughly Modern Millie | Julie Andrews | 2:46 |
| 2 | Overture: Baby Face / Do It Again! / Poor Butterfly / Stumbling / Japanese Sandman | Orchestra | 3:37 |
| 3 | Jimmy | Julie Andrews | 3:10 |
| 4 | The Tapioca | James Fox and Julie Andrews | 2:58 |
| 5 | Jazz Baby | Carol Channing | 2:46 |
| 6 | Jewish Wedding Song (Trinkt Le Chaim) | Julie Andrews | 4:02 |
| 7 | Intermission Medley: Thoroughly Modern Millie / Jimmy / Jewish Wedding Song (Trinkt Le Chaim) / Baby Face | Orchestra | 3:45 |
| 8 | Poor Butterfly | Julie Andrews | 3:33 |
| 9 | Rose of Washington Square | Ann Dee | 1:18 |
| 10 | Baby Face | Julie Andrews | 2:47 |
| 11 | Do It Again! | Carol Channing | 2:04 |
| 12 | Thoroughly Modern Millie (reprise) | Julie Andrews | 1:01 |
| 13 | Exit Music: Jazz Baby / Jimmy / Thoroughly Modern Millie | Orchestra | 2:38 |